safe OC speed is whatever the system is stable at. Unlocking the Callisto to Deneb is kinda hard. IDK how to only enable one core to get a Rana, which is more likely to be stable. On my callisto, I could get it to unlock to a stable deneb config, but the background showed artifacts. As this isn't my computer, I didn't care to OC it (it's way too powerful for a HTPC anyway). While unlocked, MTY also started ignoring my list of trips to be decoded, so it was pointless. IDK if it was a problem with the cores or the program, but I just gave up.
To unlock, you'll need to turn on Advanced Clock Calibration. If there is some form of "Hybrid" or "turbo" mode available to you, turn that on. Then, turn it to automatic, and it should unlock the extra two cores. You might play around with changing it from automatic to manual, and change the %ages from their default of -2%, but nobody knows what this actually does except make it stable, but not in most cases. Unlocking is a weird process.
As for classic overclocking, there are tutorials out there. If you have a black edition, you'll have an unlocked multiplier, and can raise/lower that from the default value to overclock just the processor, but I doubt you'll be stable at one higher than default multiplier. Instead you want to change the core frequency, which is 200 by default. Your motherboard should tell you what each BIOS thing does, so use that as a reference. To overclock my computer I have to change the frequency of the northbridge to CPU link or something like that.
What you do is steadily increase the clock speed until the system won't boot. Go ahead and set your ram to the lowest it will go for now so that the ram can't be a problem. Reset the cmos and put the clock speed slightly lower then enjoy your overclock. It's a good idea to leave it running on something intensive like mty or tripcode explorer for a few hours to test for stability. If it fails stability, then you've got to lower it more.
If you want to overvolt the processor, you can go up to a certain amount (I think 1.45 V was safe, but check other sources) and that will improve stability while decreasing the life and increasing power draw. If you go too high you will kill the processor. The RAM is tied directly to the core speed, so at 200 MHz core speed (stock speed) ddr3-1600 should run at 800 MHz DDR, or a 4:1 ratio. If you overclock to 220 MHz, the ram will run at 880 MHz, or 1760 MHz, which will probably be too much for it to handle.
Most of your OC stuff will be trial and error. Don't overvolt until you're comfortable. If it doesn't work, it doesn't work. Not all components are created equal.
"Parliamentary inquiry, Mr. Chairman - do we have to call the Gentleman a gentleman if he's not one?"